'67 Topps
This is by far my favorite set of the 60's. These were the first cards that I bought in bulk. I used to buy the 6 pack wax trays at the A&P with about every dime I could scrape together.
You should be able to buy groups of low numbers in EX+ with regularity and get a good start. The high numbers are moderately expensive but very plentiful if you are not a centering freak.
I just recently bought a couple of empty '67 wax boxes and the two style of wrappers to go with my set.
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