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Jason LThis is exactly how I collect the T206 set - by aestethic.
My subset of classic images includes a few HOFers, so please excuse those, but please consider these (Some already mentioned):
Hans Lobert (one of the very few with rich, darker tones)
Lajoie w/bat (HOF)
Keeler w/bat (HOF)
Chase, pink portrait
Nap Rucker, throwing
Liefeld, throwing (unmatched variety of colors)
Ewing (stunning sunset)
Donovan, throwing (sunset is off the hook!)
Merkle, throwing (great artistry)
Wheat (HOF)
Chappie Charles (excellent red, and a sweater)
Beals Becker (The red-white-green = xmas card)