Coincidentally, the E121 that Leon posted is the one I chose for my personal collection, but my favorite of his is the 1913 National Game/Tom Barker Game because of the price for his first non-oversized/silk/etc card. The image is great, too.
I love the National Game/Tom Barker cards a lot more than some, though. They're relatively great deals with great images and there's a decent amount in nice shape out in the wild.
If oversized is on the menu for you, his M101 Sporting News is really nice.
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