I sort my large sets by team, alphabetical order by city, National Lease first and then American League. Within a team, cards sorted by position order (P, C, 1B, 2B, 3B, SS, OF, DH), pitchers sorted by innings pitched in the last season, other positions by starter, then the backup. League Leaders, Award Winners, All-Star cards, and others all at the back. Checklists on the top.
I did it this way when I was 7, and just got so used to it that I've never changed this 'fill out the diamond for each team' order.
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