T205 for me for sure. I really do like both sets and have a 521 in t206 and complete master set in t205. I really like the card design of t205 vs t206 and the player info is fantastic!
As a set builder, I also believe the t205 set is a tougher build notwithstanding Wagner, Doyle, Plank and (to a lesser extent) Magie.
Either way you vote, both are fantastic but t205 will likely always be my favorite!!
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