I agree with the 66's being the hardest, followed by 67, 62, then 61 but don't think those 61's are nearly as hard, not easy but not as hard. 1952 is highly sought after but with an unlimited budget are much easier to find than any of those 4 60's sets. I remember it taking over a year to finish the last 5 cards in that 1966 set, every Willow Grove show and th e National couldn't find them and then finally got lucky at a show where a guy was breaking a complete set, lucky until he told me the price of those 5 "commons" but finished the hunt.
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