I love the 60's sets. If I had to pick a favorite I would say 1963, very colorful and almost HD quality photos for the time. But...
1961 is beautiful with it's unique painting/photo cards and a simple clean design
1962 is a gorgeous set in mint condition
1964 isn't as popular but it's the year I really started collecting as a kid
1965 didn't used to love it but it's really a classic design
1966 same as 1965
1967 drop dead beautiful, very little to distract from the picture
1968 hmmm, not my favorite but definitely different
1969 reminds me of 1967 set but not as cutting edge
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