I would say the E94s but there aren't enough of them out there right now so collectors would get discouraged. There needs to be eye appeal plus demand plus a decent supply. The Black Swamp cards killed the E98 set. If I had to start loading up on cards from a set because of a possible run, I would load up on T213-2 (1914) Coupons while they are still reasonably priced. The 1919 Coupons (series 3) and the series 1 cards are too rare for collectors and would only cause frustration. The M116s, E90-3s and T207s all have room to grow and increase in price but each has it's own baggage which will keep the current prices contained.
Yup, I would go for the T213-2 but keep an eye on the T210s and early Zeenut sets which have a growing number of niche collectors...
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