According to the PSA Set Registry:
Mickey Mantle - 166
Roberto Clemente - 138
Hank Aaron - 111
Willie Mays - 100
Other notables:
Nolan Ryan 87
Pete Rose 74
Cal Ripken 54
Babe Ruth - 19
Ty Cobb - 18
Honus Wagner - 3
Of course, this isn't a completely accurate picture because for some players like Ruth, most collectors usually just want 1-2 copies of that player because his cards are so expensive, so they would not attempt to collect the entire player set.
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