It's interesting that out of the first sixteen responses no one has mentioned the supposed post-war Holy Grail, 1952 Topps.
It would be hard for me to choose just one set but if I were pressed I'd probably have to go with 1953 Topps. I'd also give props to Topps for the 1958, '59, '60, '62, '63 and '71 designs as well.
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